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Bill Brodhead

WPB Enterprises Inc

Radon & Vapor Intrusion
Consultant - Researcher - Instructor
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Bill Brodhead

WPB Enterprises Inc.

Radon & Vapor Intrusion


Consultant
Researcher
Instructor
Website Info

  Home      All Info Pages     Search Website

How does Radon move in the Soil?

Multiple factors determine Radon's movement in soil

Radon movement in Soil

In general, the concentration and mobility of radon in soil are dependent on several factors, the most important of which are the soil's radium content and distribution, porosity, permeability to gas movement, and moisture content. These characteristics are, in turn, determined by the soil's parent-material composition, climate, and the soil's age or maturity. If parent-material composition, climate, vegetation, age of the soil, and topography are known, the physical and chemical properties of a soil in a given area can be predicted. As soils form, they develop distinct layers, or horizons, that are cumulatively called the soil profile. The A horizon is a surface or near-surface horizon containing a relative abundance of organic matter but dominated by mineral matter. Some soils contain an E horizon, directly below the A horizon, that is generally characterized by loss of clays, iron, or aluminum, and has a characteristically lighter color than the A horizon. The B horizon underlies the A or E horizon. Important characteristics of B horizons include accumulation of clays, iron oxides, calcium carbonate or other soluble salts, and organic matter complexes. In drier environments, a horizon may exist within or below the B horizon that is dominated by calcium carbonate, often called caliche or calcrete. This carbonate-cemented horizon is designated the K horizon in modern soil classification schemes. The C horizon underlies the B (or K) and is a zone of weathered parent material that does not exhibit characteristics of A or B horizons; that is, it is generally not a zone of leaching or accumulation. In soils formed in place from the underlying bedrock, the C horizon is a zone of unconsolidated, weathered bedrock overlying the unweathered bedrock.

Conditions of Soil that affect Radon Transport

The shape and orientation of soil particles (soil structure) control permeability and affect water movement in the soil. Soils with blocky or granular structure have roughly equivalent permeabilities in the horizontal and vertical directions, and air and water can infiltrate the soil relatively easily. However, in soils with platy structure, horizontal permeability is much greater than vertical permeability and air and moisture infiltration is generally slow. Soils with prismatic or columnar structure have dominantly vertical permeability. Platy and prismatic structures form in soils with high clay contents. In soils with shrink-swell clays, air and moisture infiltration rates and depth of wetting may be limited when the cracks in the surface soil layers swell shut. Clayrich B horizons, particularly those with massive or platy structure, can form a capping layer that impedes the escape of soil gas to the surface (Schumann and others, 1992). However, the shrinkage of clays can act to open or widen cracks upon drying, thus increasing the soil's permeability to gas flow during drier periods.

Radon Transport in Soil

Radon transport in soils occurs by two processes: (1) diffusion and (2) flow (Tanner, 1964). Diffusion is the process whereby radon atoms move from areas of higher concentration to areas of lower concentration in response to a concentration gradient. Row is the process by which soil air moves through soil pores in response to differences in pressure within the soil or between the soil and the atmosphere, carrying the radon atoms along with it. Diffusion is the dominant radon transport process in soils of low permeability, whereas flow tends to dominate in highly permeable soils (Sextro and others, 1987). In low-permeability soils, much of the radon may decay before it is able to enter a building because its transport rate is reduced. Conversely, highly permeable soils, even those that are relatively low in radium, such as those derived from some types of glacial deposits, have been associated with high indoor radon levels in Europe and in the northern United States (Akerblom and others, 1984; Kunz and others, 1989; Sextro and others, 1987).

Karst Geology

In areas of karst topography formed in carbonate rock (limestone or dolomite) environments, solution cavities and fissures can increase soil permeability at depth by providing additional pathways for gas flow. Homes in hilly limestone regions of the southern Appalachians were found to have higher indoor radon concentrations during the summer than in the winter. A suggested cause for this phenomenon involves temperature/pressure-driven flow of radon-laden air from subsurface solution cavities in the carbonate rock into houses. As warm air enters solution cavities that are higher on the hill slope than the homes, it cools and settles, pushing radon-laden air from lower in the cave or cavity system into structures on the hill slope (Gammage and others, 1993). In contrast, homes built over caves having openings situated below the level of the home had higher indoor radon levels in the winter, caused by cooler outside air entering the cave, driving radon laden air into cracks and solution cavities in the rock and soil, and ultimately, into homes (Gammage and others, 1993). USGS Open-File Report

Radon Movement in Soil and Soil Moisture affect

Not all radium contained in soil grains and grain coatings will result in mobile radon when the radium decays. Depending on where the radium is distributed in the soil, many of the radon atoms may remain imbedded in the soil grain containing the parent radium atom, or become imbedded in adjacent soil grains. The portion of radium that releases radon into the pores and fractures of rocks and soils is called the emanating fraction. When a radium atom decays to radon, the energy generated is strong enough to send the radon atom a distance of about 40 nanometers (1 nm = 10~9 meters), or about 2xlO~6 inches this is known as alpha recoil (Tanner, 1980). Moisture in the soil lessens the chance of a recoiling radon atom becoming imbedded in an adjacent grain. Because water is more dense than air, a radon atom will travel a shorter distance in a waterfilled pore than in an air-filled pore, thus increasing the likelihood that the radon atom will remain in the pore space. Intermediate moisture levels enhance radon emanation but do not significantly affect permeability. However, high moisture levels can significantly decrease the gas permeability of the soil and impede radon movement through the soil.

Radon Concentrations in the Soil

Concentrations of radon in soils are generally many times higher than those inside of buildings, ranging from tens of pCi/L to more than 100,000 pCi/L, but typically in the range of hundreds to low thousands of pCi/L. Soil-gas radon concentrations can vary in response to variations in climate and weather on hourly, daily, or seasonal time scales. Schumann and others (1992) and Rose and others (1988) recorded order-of-magnitude variations in soil-gas radon concentrations between seasons in Colorado and Pennsylvania. The most important factors appear to be (1) soil moisture conditions, which are controlled in large part by precipitation; (2) barometric pressure; and (3) temperature. Washington and Rose (1990) suggest that temperature-controlled partitioning of radon between water and gas in soil pores also has a significant influence on the amount of mobile radon in soil gas.

Source:

THE USGS/EPA RADON POTENTIAL ASSESSMENTS: AN INTRODUCTION by Linda C.S. Gundersen and R. Randall Schumann U.S. Geological Survey and Sharon W. White U.S. Environmental Protection Agency 1993 .

How does Radon
move in the Soil?

Multiple factors determine Radon's
movement in soil

Radon Movement in Soil

In general, the concentration and mobility of radon in soil are dependent on several factors, the most important of which are the soil's radium content and distribution, porosity, permeability to gas movement, and moisture content. These characteristics are, in turn, determined by the soil's parent-material composition, climate, and the soil's age or maturity. If parent-material composition, climate, vegetation, age of the soil, and topography are known, the physical and chemical properties of a soil in a given area can be predicted. As soils form, they develop distinct layers, or horizons, that are cumulatively called the soil profile. The A horizon is a surface or near-surface horizon containing a relative abundance of organic matter but dominated by mineral matter. Some soils contain an E horizon, directly below the A horizon, that is generally characterized by loss of clays, iron, or aluminum, and has a characteristically lighter color than the A horizon. The B horizon underlies the A or E horizon. Important characteristics of B horizons include accumulation of clays, iron oxides, calcium carbonate or other soluble salts, and organic matter complexes. In drier environments, a horizon may exist within or below the B horizon that is dominated by calcium carbonate, often called caliche or calcrete. This carbonate-cemented horizon is designated the K horizon in modern soil classification schemes. The C horizon underlies the B (or K) and is a zone of weathered parent material that does not exhibit characteristics of A or B horizons; that is, it is generally not a zone of leaching or accumulation. In soils formed in place from the underlying bedrock, the C horizon is a zone of unconsolidated, weathered bedrock overlying the unweathered bedrock.

Conditions of Soil that affect Radon Transport

The shape and orientation of soil particles (soil structure) control permeability and affect water movement in the soil. Soils with blocky or granular structure have roughly equivalent permeabilities in the horizontal and vertical directions, and air and water can infiltrate the soil relatively easily. However, in soils with platy structure, horizontal permeability is much greater than vertical permeability and air and moisture infiltration is generally slow. Soils with prismatic or columnar structure have dominantly vertical permeability. Platy and prismatic structures form in soils with high clay contents. In soils with shrink-swell clays, air and moisture infiltration rates and depth of wetting may be limited when the cracks in the surface soil layers swell shut. Clayrich B horizons, particularly those with massive or platy structure, can form a capping layer that impedes the escape of soil gas to the surface (Schumann and others, 1992). However, the shrinkage of clays can act to open or widen cracks upon drying, thus increasing the soil's permeability to gas flow during drier periods.

Radon Transport in Soil

Radon transport in soils occurs by two processes: (1) diffusion and (2) flow (Tanner, 1964). Diffusion is the process whereby radon atoms move from areas of higher concentration to areas of lower concentration in response to a concentration gradient. Row is the process by which soil air moves through soil pores in response to differences in pressure within the soil or between the soil and the atmosphere, carrying the radon atoms along with it. Diffusion is the dominant radon transport process in soils of low permeability, whereas flow tends to dominate in highly permeable soils (Sextro and others, 1987). In low-permeability soils, much of the radon may decay before it is able to enter a building because its transport rate is reduced. Conversely, highly permeable soils, even those that are relatively low in radium, such as those derived from some types of glacial deposits, have been associated with high indoor radon levels in Europe and in the northern United States (Akerblom and others, 1984; Kunz and others, 1989; Sextro and others, 1987).

Karst Geology

In areas of karst topography formed in carbonate rock (limestone or dolomite) environments, solution cavities and fissures can increase soil permeability at depth by providing additional pathways for gas flow. Homes in hilly limestone regions of the southern Appalachians were found to have higher indoor radon concentrations during the summer than in the winter. A suggested cause for this phenomenon involves temperature/pressure-driven flow of radon-laden air from subsurface solution cavities in the carbonate rock into houses. As warm air enters solution cavities that are higher on the hill slope than the homes, it cools and settles, pushing radon-laden air from lower in the cave or cavity system into structures on the hill slope (Gammage and others, 1993). In contrast, homes built over caves having openings situated below the level of the home had higher indoor radon levels in the winter, caused by cooler outside air entering the cave, driving radon laden air into cracks and solution cavities in the rock and soil, and ultimately, into homes (Gammage and others, 1993). USGS Open-File Report

Radon Movement in Soil and Soil Moisture affect

Not all radium contained in soil grains and grain coatings will result in mobile radon when the radium decays. Depending on where the radium is distributed in the soil, many of the radon atoms may remain imbedded in the soil grain containing the parent radium atom, or become imbedded in adjacent soil grains. The portion of radium that releases radon into the pores and fractures of rocks and soils is called the emanating fraction. When a radium atom decays to radon, the energy generated is strong enough to send the radon atom a distance of about 40 nanometers (1 nm = 10~9 meters), or about 2xlO~6 inches this is known as alpha recoil (Tanner, 1980). Moisture in the soil lessens the chance of a recoiling radon atom becoming imbedded in an adjacent grain. Because water is more dense than air, a radon atom will travel a shorter distance in a waterfilled pore than in an air-filled pore, thus increasing the likelihood that the radon atom will remain in the pore space. Intermediate moisture levels enhance radon emanation but do not significantly affect permeability. However, high moisture levels can significantly decrease the gas permeability of the soil and impede radon movement through the soil.

Radon Concentrations in the Soil

Concentrations of radon in soils are generally many times higher than those inside of buildings, ranging from tens of pCi/L to more than 100,000 pCi/L, but typically in the range of hundreds to low thousands of pCi/L. Soil-gas radon concentrations can vary in response to variations in climate and weather on hourly, daily, or seasonal time scales. Schumann and others (1992) and Rose and others (1988) recorded order-of-magnitude variations in soil-gas radon concentrations between seasons in Colorado and Pennsylvania. The most important factors appear to be (1) soil moisture conditions, which are controlled in large part by precipitation; (2) barometric pressure; and (3) temperature. Washington and Rose (1990) suggest that temperature-controlled partitioning of radon between water and gas in soil pores also has a significant influence on the amount of mobile radon in soil gas.

Source:

THE USGS/EPA RADON POTENTIAL ASSESSMENTS: AN INTRODUCTION by Linda C.S. Gundersen and R. Randall Schumann U.S. Geological Survey and Sharon W. White U.S. Environmental Protection Agency 1993 .

Radon mitigation call Integra Environmental 610 346-8004
For consulting Bill 484 626-0993 - © 2021 Bill Brodhead

For Radon System estimates or Fan repairs call
Integra Environmental at 610- 346-8004
© 2021 Bill Brodhead

For consulting call Bill at 484 626-0993